Ab-initio Quantum Transport with the GW Approximation, 42,240 Atoms, and Sustained Exascale Performance

The work

TitleAb-initio Quantum Transport with the GW Approximation, 42,240 Atoms, and Sustained Exascale Performance
AuthorsNicolas Vetsch; Alexander Maeder; Vincent Maillou; Anders Winka; Jiang Cao; Grzegorz Kwaśniewski; Leonard Deuschle; Torsten Hoefler; Alexandros Nikolaos Ziogas; Mathieu Luisier
Typeconference paper
Year2025
Citekeyvetsch2025abinitio

Where it appeared

Published inProceedings of the International Conference for High Performance Computing, Networking, Storage and Analysis (SC '25)
PublisherAssociation for Computing Machinery
Pages1--13

Identifiers

DOI10.1145/3712285.3771784
arXiv2508.19138
OpenAlexW4416203768

Access

Landing pagehttps://doi.org/10.1145/3712285.3771784
Free full texthttps://doi.org/10.1145/3712285.3771784

Abstract

Designing nanoscale electronic devices such as the currently manufactured nanoribbon field-effect transistors (NRFETs) requires advanced modeling tools capturing all relevant quantum mechanical effects. State-of-the-art approaches combine the non-equilibrium Green's function (NEGF) formalism and density functional theory (DFT). However, as device dimensions do not exceed a few nanometers anymore, electrons are confined in ultra-small volumes, giving rise to strong electron-electron interactions. To account for these critical effects, DFT+NEGF solvers should be extended with the GW approximation, which massively increases their computational intensity. Here, we present the first implementation of the NEGF+GW scheme capable of handling NRFET geometries with dimensions comparable to experiments. This package, called QuaTrEx, makes use of a novel spatial domain decomposition scheme, can treat devices made of up to 84,480 atoms, scales very well on the Alps and Frontier supercomputers (> 80% weak scaling efficiency), and sustains an exascale FP64 performance on 42,240 atoms (1.15 Eflop/s).

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Where it came fromhttps://doi.org/10.1145/3712285.3771784

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Cite it as

@inproceedings{vetsch2025abinitio,
  title = {Ab-initio Quantum Transport with the GW Approximation, 42,240 Atoms, and Sustained Exascale Performance},
  author = {Nicolas Vetsch and Alexander Maeder and Vincent Maillou and Anders Winka and Jiang Cao and Grzegorz Kwaśniewski and Leonard Deuschle and Torsten Hoefler and Alexandros Nikolaos Ziogas and Mathieu Luisier},
  year = {2025},
  booktitle = {Proceedings of the International Conference for High Performance Computing, Networking, Storage and Analysis (SC '25)},
  pages = {1--13},
  publisher = {Association for Computing Machinery},
  doi = {10.1145/3712285.3771784},
  url = {https://doi.org/10.1145/3712285.3771784},
}

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